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學術成果

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論文內容
論文分類碩士論文
學號10125602
姓名顏如慧
標題(中)電觸媒技術去除水中大腸桿菌之研究
標題(英)Study on the removal of Escherichia coli by Electrocatalyst technology in the water
指導教授章日行
畢業日期2014-08
附件檔案 
參考連結http://ndltd.ncl.edu.tw/cgi-bin/gs32/gsweb.cgi?o=dnclcdr&s=id=%22102CYUT0087004%22.&searchmode=basic&extralimit=asc=%22%E6%9C%9D%E9%99%BD%E7%A7%91%E6%8A%80%E5%A4%A7%E5%AD%B8%22&extralimitunit=%E6%9C%9D%E9%99%BD%E7%A7%91%E6%8A%80%E5%A4%A7%E5%AD%B8
摘要在各類飲用水水質及水源上,環保署及衛生署針對大腸桿菌訂定法規標準,而一般飲用水通常使用逆滲透(Reverse Osmosis)、臭氧及紫外線殺菌,其分別具有不同缺點。本研究利用電觸媒處理技術快速去除水中之大腸桿菌,並探討不同操作條件下之最佳可行性。電觸媒技術(Electrocatalyst)為目前新穎廢水處理技術之一,其利用一外加電場提供能量於觸媒材料,進而於觸媒材料上產生具有強氧化作用之氫氧自由基。此處理技術的優點包括易破壞細胞膜、能分解有機污染物及去除色度等,所以,本研究冀望能利用此技術達到水中滅菌的
參考文獻Abongo, B. O., and Maggy, N. B.,“Prevalence and characterization of Escherichia coli O157:H7 isolates from meat and meat products sold in Amathole District, Eastern Cape Province of South Africa,” Food Microbiology, Vol. 26, pp. 173-176 (2009)Bougeard, C. M. M., Goslan, E. H., Jefferson, B., and Parsons, S. A., “Comparison of the disinfection by-product formation potential of treated waters exposed to chlorine and monochloramine,” Water Research, Vol. 44, pp. 729–740(2010)Cálix-Lara, T. F., Rajendran, M., Talcott, S. T., Smith, S. B., Miller, R. K., Castillo, A., Sturino, J. M., and Taylor, T. M., “Inhibition of Escherichia coli O157:H7 and Salmonella enterica on spinach and identification of antimicrobial substances roduced by a commercial Lactic Acid Bacteria food safety intervention,” Food Microbiology , Vol. 38,pp.192-200(2014)Chang, J. H., Ellis, A. V., Hsieh, Y. H., Tung, C. H., and Shen, S. Y., “Electrocatalytic characterization and dye degradation of Nano-TiO2 electrode films fabricated by CVD,” Science of the Total Environment, Vol. 407, pp. 5914-5920 (2009)Chang, J. H., Yang, T. J., and Tung, C. H., “Performance of nano- and nonnano-catalytic electrodes for decontaminating municipal wastewater,” Journal of Hazardous Materials, Vol. 163, pp. 152-157 (2009)Cho, M., Chung, H., Choi, W., and Yoon, J., “Linear correlation between inactivation of E. coli and OH radical concentration in TiO2 photocatalytic disinfection” Water Research, Vol. 38, pp. 1069-2077(2004).Cui, Y. H., Li, X. Y., and Chen, G. H., “Electrochemical degradation of bisphenol A on different anodes,” Water research, Vol. 43, pp. 1968-1976 (2009)Dostanić, J., Grbić, B., Radić, N., Stojadinović, S., Vasilić, R., and Vuković, Z., “Preparation and photocatalyic properties of TiO2-P25 film prepared y spray pyrolysis method, ” Applied Surface Science, Vol. 274, pp. 321–327(2013)Giornelli, T., Löfberg , A., and Bordes-Richard, E., “Preparation and characterization of VOx/TiO2 catalytic coatings on tainless steel plates for structured catalytic reactors, ” Applied Catalysis A: General, Vol. 305, pp. 197–203 (2006)Guzel-Seydim, Z. B., Greene, A. K., and Seydim, A. C., “Use of ozone in the food industry” Lebensm.-Wiss. u.-Technol, Vol. 37, pp. 453–460(2004)Halliwell, B., and Gutterridge, J. M. C., “Free radicals in biology and medicine” Clarendon Press, Oxford, 2nd ed., pp. 30(1989).Huang, D., Miyamoto, Y., Matsumoto, T., Tojo, T., Fan, T., Ding, J., Guo, Q., and Zhang, D., “Preparation and characterization of high-surface-area TiO2/activated carbon by low-temperature impregnation, ” Separation and Purification Technology, Vol. 78, pp. 9–15(2011)Hussain, S. N., Heras, N., Asghar, H. M. A., Brown, N. W., and Roberts, E. P. L., “Disinfection of water by adsorption combined with electrochemical treatment, ”Water Research, Vol. 54, pp. 170 -178(2014)Kurzweil, P., HISTORY Electrochemistry, Reference Module in Chemistry, Germany, pp. 533-554(2009)Li, Y., Wang, F., Zhou, G., and Ni, Y., “Aniline degradation by electrocatalytic oxidation,” Chemosphere, Vol. 53, pp. 1229–1234(2003)Linsebigler, A.L., Lu, G., and Yates Jr, J.T., “Photocatalysis on TiO2 surface: principles, mechanism, and selected results” Chemical Reviews, Vol. 95, pp. 735-758(1995).Lissens, G., Pieters, J., Verhaege, M., Pinoy, L., and Verstraete, W., “Electrochemical degradation of surfactants by intermediates of water discharge at carbon-based electrodes, ” Electrochimica Acta, Vol. 48, pp. 1655-1663(2003)López, N., Gómez-Segura, J., Marín, R. P., and Pérez-Ramírez, J., “Mechanism of HCl oxidation (Deacon process) over RuO2, ” Journal of Catalysis, Vol. 255, pp. 29–39(2008)Low, D., Hamood, A., Rei, T., Mosley, T., Tran, P., Song, L., and Morse, A., “Attachment of selenium to a reverse osmosis membrane to inhibit biofilm formation of S. aureus,” Journal of Membrane Science, Vol. 378, pp. 171-178(2011)Mohan, N., and Balasubramanian, N., “In situ electrocatalytic oxidation of acid violet 12 dye effluent, ” Journal of Hazardous Materials, Vol. B136, pp. 239–243(2006)McCloskey, D., Palsson1, B., and Feist, A. M., “Basic and applied uses of genome-scale metabolic network reconstructions of Escherichia coli”, EMBO and Macmillan Publishers Limited, USA, pp.661(2013)Mainil, J., “Escherichia coli virulence factors, ” Veterinary Immunology and Immunopathology, Vol. 152, pp. 2–12(2013)Neupane, M., Abu-Ali, G. S., Lacher,D. W., Manning, S. D., and Riordan, J. T., “Shiga toxin 2 overexpression in Escherichia coli O157:H7 strains associated with severe human disease” Microbial Pathogenesis, Vol. 51, pp. 466-470(2011)Ning, P., Bart, H.-J., Jiang, Y., Haan, A.D., and Tien, C., “Treatment of organic pollutants in coke plant wastewater by the method of ultrasonic irradiation, catalytic oxidation and activated sludge” Separation and Purification Technology, Vol. 41, pp. 133-139(2005).Pangarkar, V.G., Bhatkhande, D.S., Kamble, S.P., and Sawant, S.B., “Photocatalytic and photochemical degradation of nitrobenzene using artificial ultraviolet light” Chemical Engineering Journal, Vol. 102, pp. 283-290(2004).Panizza, M., and Cerisola, G., “Electrocatalytic materials for the electrochemical xidation of synthetic dyes, ” Applied Catalysis B: Environmental , Vol. 75, pp. 95–101(2007)Park, Y. H., Uhm, H. S., Lee, H. Y., Lee, P. C., and Hong, Y. F., “Sterilization effects of ozone decay time in acidic water against Bacillus atrophaeus endospores,” New Biotechnology, Vol. 25S, pp. S198(2009)Pascual, A., Llorca, I., and Canut, A., “Use of ozone in food industries for reducing the environmental impact of cleaning and disinfection activities, ” Trends in Food Science & Technology, Vol. 18, pp. S29-S35(2007)Parsons, S., “Advanced oxidation processes for water and wastewater treatment” IWA Publishing, UK, pp. 4(2004).Oliveira, G. R. d., Fernandes, N. S., Melo, J. V. d., Silva, D. R. d., Urgeghe, C., Martínez-Huitle, C. A., “Electrocatalytic properties of Ti-supported Pt for decolorizing and removing dye from synthetic textile wastewaters,” Chemical Engineering Journal, Vol. 168, pp. 208–214(2011)Quan, X., Cheng, Z., Chen, B., and Zhu, X., “Electrochemical oxidation of recalcitrant organic compounds in biologically treated municipal solid waste leachate in a flow reactor,” Journal of Environmental Sciences, Vol. 25(10), pp. 2023–2030(2013)Roccaforte, F., Giannazzo, F., Iucolano, F., Eriksson, J., Weng, M. H., and Raineri, V., “Surface and interface issues in wide band gap semiconductor electronics, ” Applied Surface Science, Vol. 256, pp. 5727–5735(2010)Sanz, M., Rebollar, E., Ganeev, R. A., and Castillejo, M., “Nanosecond laser-induced periodic surface structures on wide band-gap semiconductors, ” Applied Surface Science, Vol. 278, pp. 325–329(2013)Su, J., Lu, N., Zhao, J., Yu, H., Huang, H., Dong, X., Quan, X., “Nano-cubic structured titanium nitride particle films as cathodes for the effective electrocatalytic debromination of BDE-47, ” Journal of Hazardous Materials, Vol. 231–232, pp. 105–113(2012)Tian, F., Qiang, Z., Liu, W., and Ling, W., “Methiocarb degradation by free chlorine in water treatment: Kinetics and pathways, ” Chemical Engineering Journal, Vol. 232, pp. 10–16(2013)Würtele, M. A., Kolbe, T., Lipsz, M., Külberg, A., Weyers, M., Kneissl, M., and Jekel, M., “Application of GaN-based ultraviolet-C light emitting diodese UV LEDse for water disinfection,” water research, Vol. 45, pp. 1481-1489(2011)Yang, D., and Englehardt, J. D., “Electrochemical oxidation for landfill leachate treatment, ” Waste Management, Vol. 27, Issue. 3, pp. 380–388(2007)Yang, X., Guo, W., and Lee, W., “Formation of disinfection byproducts upon chlorine dioxide preoxidation followed by chlorination or chloramination of natural organic matter, ” Chemosphere, Vol. 91, pp. 1477–1485(2013)Zhou, M., Särkkä, H., and Sillanpää, M., “A comparative experimental study on methyl orange degradation by electrochemical oxidation on BDD and MMO electrodes, ” Separation and Purification Technology, Vol. 78, pp. 290–297(2011)Zhong, Y., Liang, X., He, Z., Tan, W., Zhu, J., Yuan, P., Zhu, R., He, H., “The constraints of transition metal substitutions (Ti, Cr, Mn, Co andNi) in magnetite on its catalytic activity in heterogeneous Fentonand UV/Fenton reaction: From the perspective of hydroxylradical generation, ” Applied Catalysis B: Environmental, Vol. 150-151, pp.612–618(2014)中文文獻王飛龍,“觸媒化學” 滄海書局,第2-145頁,臺中市(2012)王淑娟,“液相光催化反應之氫氧自由基生成量測-以甲醇為自由基捕捉劑” ,碩士論文, 國立高雄第一科技大學環境與安全衛生工程系,高雄(2006)石濤,“環境微生物”鼎茂圖書出版股份有限公司,第70-83頁,台北市(2009)沈善鎰,“製備奈米二氧化鈦觸媒材料與應用電觸媒處理染料廢水”,碩士論文,朝陽科技大學環境工程與管理研究所,台中市(2008)林永璋,“以臭氧/紫外光程序去除以二胺四乙酸之研究”,碩士論文,國立中山大學環境工程研究所,高雄(2003)林奎君,“利用TEM-STM方法研究單根二氧化釕奈米線之導電性質”,碩士論文,國立清華大學工程與系統科學系,新竹(2006)林哲民,“以染料A07探討Fenton程序升成自由基之研究”,碩士論文,國立雲林科技大學環境與安全衛生工程系,雲林(2012)馬振基,“奈米材料科技原理與應用”,全華科技,第-頁,臺北市(2004)唐政宏,“探討二氧化鈦觸媒電極氫氧自由基產率及處理生活污水效率”,碩士論文,朝陽科技大學環境工程與管理研究所,台中市(2007)許洋銘,“電觸媒應用於鑄幣廠及印刷廠廢水之研究”,碩士論文,朝陽科技大學環境工程與管理研究所,台中市(2012)許家綺,“探討光電觸媒之氫氧自由基檢測方法及其產率”,碩士論文,朝陽科技大學環境工程與管理研究所,台中市(2011)彭章娥、吳峰、鄭南聖,“光照下銅離子對水中氫氧自由基生成量的影響”,環境科學與技術學報,武漢大學資源與環境學院,第29卷第4期2006年4月菊地正典,“圖解半導體”世茂出版社,第26-39頁,台北縣(2005)楊蘭芳,“液相光催化反應之氫氧自由基生成量測-以二甲基亞碸為自由基捕捉劑”,碩士論文,國立高雄第一科技大學環境與安全衛生工程所,高雄(2006)鄭佳倩,“以自由基捕捉/螢光法量測光催化反應中氫氧自由基之生成”,碩士論文,國立高雄第一科技大學環境與安全衛生工程系,高雄(2007)藤嶋昭、橋本和仁、渡部俊也,“圖解光觸媒”世茂出版社,第110-117頁,台北縣(2006)

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