:::

學術成果

:::
論文內容
論文分類碩士論文
學號9025608
姓名廖盈智
標題(中)循環改良式電動力系統之電化學反應
標題(英)The Study on Electrochemical Reactions in a Circulation-Enhanced Electrokinetic
指導教授章日行
畢業日期2003-07
附件檔案 
參考連結http://ir.lib.cyut.edu.tw:8080/handle/310901800/1663
摘要本研究設計一組改良式電動力系統,以聚氯乙烯 (PVC) 製作規格為長20 cm ´寬8 cm ´高10 cm的電動力系統槽體,並配合連通原理與循環裝置的使用,主要目的是為了避免電動力反應進行中土壤產生酸化的問題,並希望得到穩定的電動力處理系統。此外,藉由改變相關操作參數以求了解系統中的反應與變化,研究的控制因子包含:電解質種類、電解質操作液濃度、操作電壓梯度、電極板種類與電極板配製位置。 依據實驗結果分析本循環改良式電動力系統適當的操作條件如下:以0 01 M碳酸根鹽類電解質作為電動力系統之操作溶液,外加
參考文獻Acar, Y. B., and Alshawabkeh, A. N., “Electrokinetic Remediation. I. Pilot-Scale Tests with Lead-Spiked Kaolinite,” Journal of Geotechnical Engineering, Vol. March, pp. 173-185 (1996).
Acar, Y. B., and Alshawabkeh, A. N., “Principles of Electrokinetic Remediation,” Environmental Science & Technology, Vol. 27, No. 13, pp. 2638-2647 (1993).
Acar, Y. B., and Haider, L., “Transport of Low-Concentration Contaminants in Saturated Earthen Barriers,” Journal of Geotechnical Engineering, Vol. 116, No. 7, pp. 1031-1052 (1990).
Acar, Y. B., Gale, R. J., Alshawabkeh, A. N., Marks, R. E., Puppala, S., Bicka, M., and Parker, R., “Electrokinetic Remediation: Basics and Technology Status,” Journal of Hazardous Materials, Vol. 40, No. 2, pp. 117-137 (1995).
Acar, Y. B., Hame, J. T., Alshawabkeh, A. N., and Gale, R. J., “Removal of Cadmium from Saturated Kaolinite by the Application of Electrical Current,” Geotechnique, Vol. 44, No. 2, pp. 239-254 (1994).
Acar, Y. B., Hamed, J. T., and Gale, R. J., “Removal of Cadmium (II) from Saturated Kaolinite by the Application of Electrical Current,” Geotechnique, Vol. 44, No. 2, pp. 239-254 (1994).
Acar, Y. B., Lee, H., and Gale, R. J., “Phenol Removal from Kaolinite by Electrokinetics,” Journal of Geotechnical Engineering, Vol. 118, pp. 1837-1852 (1992).
Acar, Y. B., Ozsu, E. E., Alshawabkeh, A. N., Rabbi, M. F., and Gale. R. J., “Enhance Soil Bioremediation with Electric Fields,” Chemtech, Vol. 26, No. 4, pp. 40-44 (1996).
Brain, E. R., Berg, M. T., Thompson, J. C., and Hatfield, J. H., “Chemical Conditioning of Electrode Reservoirs during Electrokinetic Soil Flushing of Pb-Contaminated Silt Loam,” Journal of Environmental Engineering, Vol. 121, No. 11, pp. 805-815 (1995).
Bruell, C. J., Segall, B. A., and Walsh, M. T, “Electro-Osmosis Removal of Gasoline Hydrocarbons and TCE from Clay,” Journal of Environmental Engineering, Vol. 118, No. 1, pp.68-83 (1992).
Butterfield, R., and Johnson, I. W., “The Influence of Electroosmosis on Metallic Piles in Clay,” Geotechnique, Vol. 30, pp. 17-38 (1980).
Casagrande, L., “Electro-Osmosis in Soils,” Geotechnique, Vol. 1, No. 1, pp. 1959-1977 (1949).
Chang, J. H., Qiang, Z., Huang, C. P., and Cha, D., “Electroosmotic Flow Rate: A Semiempirical Approach,” Chapter 15 in Nuclear Site Remediation: First Accomplishments of the Environmental Management Science Program, ACS Symposium Series, Vol. 778, pp. 247-266 (2000).
Chilingar, G. V., Loo, W. W., Khilyuk, L. F., and Katz, S. A., “Electrobioremediation of Soils: Progress Report,” Energy Sources, Vol. 19, pp. 129-146 (1997).
Hamed, B. J., Acar, Y. B., and Gale, R. J., “Pb (II) Removal from Kaolinite by Electrokinetics,” Journal of Geotechnical Engineering, Vol. 117, No. 2, pp. 241-271 (1991).
Hamed, J. T., and Bhadra, A., “Influence of Current Density and pH on Electrokinetics,” Journal of Hazardous Materials, Vol. 55, pp. 279-294 (1997).
Hansen, H. K., Ottosen, L. M., Laursen, S. and Villumsen, A., “Electrodialytic Remediation of Soils Polluted with Cu, Cr, Hg, Pb, and Zn,” Journal of Chemical Technology and Biotechnology, Vol. 70, No. 1, pp. 67-73 (1997).
Ho, V. S., “The Lasagna Technology for in Situ Soil Remediation. 1. Small Field Test,” Environmental Science & Technology, Vol. 33, No. 7, pp. 1086-1091 (1999).
Jacob, H. M., Electrokinetic Transport Phenomena, AOSTRA, Canada (1994).
Kim, J., and Lee, K., “Effects of Electric Field Directions on Surfactant Enhanced Electrokinetic Remediation of Diesel-Contaminated Sand Column,” Journal of Environmental Science and Health, Vol. 34, No. 4, pp. 863-877 (1999).
Lee, H. H., and Yang, J. W., “A New Method to Control Electrolytes pH by Circulation System in Electrokinetic Soil Remediation,” Journal of Hazardous Materials, Vol. B77, pp. 227-240 (2000).
Leinz, R. W., Hoover, D. B., and Meier, A. L., “NEOCHIN: An Electrochemical Method for Environmental Application,” Journal of Geochemical Exploration, Vol. 64, No. 3, pp. 421-434 (1998).
Li, Z., Yu, J. W., and Neretnieks, I., “Electroremediation: Removal of Heavy Metals from Soils by Using Cation Selective Membrane,” Environmental Science & Technology, Vol. 32, pp. 394-397 (1998).
Li, Z., Yu, J. W., and Neretnieks, I., “Removal of Pb (II), Cd (II), and Cr (III) from sand by Electromigration,” Journal of Hazardous Materials, Vol. 55, No. 1-3, pp. 295-304 (1997).
Mitchell, J. K., “Condition Phenomena: from Theory to Geotechnical Practice,” Geotechnique, Vol. 41, No. 3, pp. 299-340 (1991).
Mitchell, J. K., Fundamentals of Soil Behavior, 2nd edition, John Wiley & Sons, New York (1993).
Nycr, E. K., Fam, S., Kidd, D. F., Palmcr, P. L., Bocttcheer, G., Crossman, T. L., and Suthersan, S. S., In-Situ Treatment, CRC Press Inc., pp. 310-314 (1996).
Oldham, K. B. and Myland, J. C., Fundamentals of Electrochemical Science, Academic Press Inc., California (1993).
Pamukcu, S., “Electro-Chemical Technologies for In-Situ Restoration of Contaminated Subsurface Soils,” Electronic Journal of Geotechnical Engineering, Vol. 2 (1997). http://www.ejge.com/1997/Ppr9704/Abs9704.htm
Popov. K., Yachmenev, V., Kolosov, A., and habanova, N., “Effect of Electroosmotic Flow Enhancement by Chelatig Reagents,” Colloids and Surfaces A: Physicochemical and Engineering Aspects, Vol. 160, pp. 135-140 (1999).
Probstein, R. F., and Hicks, R. E., “Removal of Contaminants from Soils by Electric Fields,” Science, Vol. 260, pp. 498-503 (1993).
Puppala, K. S., Alshawabkeh, A. N., Acar, Y. B., Gale, R, J., and Bricka, M., “Enhanced Electrokinetic Remediation of High Sorption Capacity Soil,” Journal of Hazardous Meterials, Vol. 55, PP. 221-237 (1997).
Reddy, K. R., and Chinthamreddy, S., “Electrokinetic Remediation of Heavy Metal-Contaminated Soils under Reducing Environments,” Waste Management, Vol. 19, pp. 269-282 (1999).
Reiger, P. H., Electrochemistry, 2nd edition, Chapman & Hall, New York, p.445 (1994)
Sah, J. G., and Chen, J. Y., “Study of the Electrokinetic Process on Cd and Pb Spiked Soils,” Journal of Hazardous Materials, Vol. 58, pp. 301-315 (1998).
Saichek, R. E., and Reddy, K. R., “Effect of pH Control at the Anode for the Electrokinetic Removal of Phenanthrene from Kaolin Soil,” Chemosphere, Vol. 51, pp. 273-287 (2003).
Sawyer, C. N., McCarty, P L., and Parkin, G. F., Chemistry for Environmental Engineering, 4th edition, McGraw-Hill, Singapore, pp. 332-334 (1994).
Shapiro, A. P., and Probstein, R. F., “Removal of Contaminants from Saturated Clay by Electroosmosis,” Environmental Science & Technology, Vol. 27, No. 2, pp. 283-291 (1993).
Shapiro, A. P., Renaud, P. C., and Probstein, R. F., “Preliminary Studies on the Removal of Chemical Species from Saturated Porous Media by Electroosmosis,” Physicochemical Hydrodynamics, Vol. 11, No. 5-6, pp. 785-802 (1989).
Takiyama, L., and Huang, C. P., “In-Situ Removal of Phenols from Contaminated Soil by Electro-Osmosis Process,” Proceeding of 27th Mid-Atlantic Industrial & Hazardous Waste Conference, Lehigh U., Technomic, Pub. Co, Lancaster, PA. Pp. 835-846 (1995).
Trombly, J., “Electrochemical Remediation Takes to the Field,” Environmental Science & Technology, Vol. 28, No. 6, pp. 289A-291A (1994).
Van Olphen, H., An Introduction to Clay Colloid Chemistry, 2nd edition, John Wiley & Sons, New York (1977).
Vane, M. L., and Zang, G. M., “Effects of Aqueous Phase Properties on Clay Particle Zeta Potential and Electro-osmotic Permeability: Implications for Electro-kinetic Soil Remediation Processes,” Journal of Hazardous Materials, Vol. 55, No. 3, pp. 1-22 (1997).
Yang, G. C. C., and Liu, C. Y., “Removal of TCE Contaminated Soils by in situ EK-Fenton Process,” Journal of Hazardous Materials, Vol. 85, No. 3, pp. 317-331 (2001).
Yang, G. C. C., and Long, Y. W., “Removal and Degradation of Phenol in a Saturated Flow by In-Situ Electrokinetic Remediation and Fenton-Like Process,” Journal of Hazardous Materials, Vol. 69, No. 3, pp. 259-271 (1999).
Yeung, A. T., “Coupled Flow Equations for Water, Electricity, and Ionic contaminants Through Clayey Soils under Hydraulic, Electrical and Chemical Gradient,” Journal of Non-Equilibrium Thermodynamics, Vol. 15, No. 3, pp. 247-267 (1990).
Yeung, A. T., “Electrokinetic Flow Prow Processes in Porous Media and Their Applications, in: Advances in Porous Media, Corapcioglu, M. Y. (Ed.),” Elsevier, Amsterdam, The Netherlands, Vol.2, pp. 309-395 (1994).
Yeung, A. T., and Mitchell, J. K., “Coupled Fluid, Electrical, and Chemical Flow in Soils”, Geotechnique, Vol. 43, No. 1, pp. 121-134 (1993).
Yeung, A. T., Hsu, C. N., and Menon, R. M., “EDTA-Enhanced Electrokinetic Extraction,” Journal of Environment Engineering, Vol. 122, No. 8, pp. 666-673 (1996).
Yeung, A. T., Hsu, C. N., and Menon, R. M., “Physicochemical Soil-contaminant Interactions during Electrokinetic Extraction,” Journal of Hazardous Materials, Vol. 55, pp. 221-237 (1997).
Yeung, A. T., Hsu, C., and Menon, R. M., “EDTA-Enhanced Electrokinetic Extraction,” Journal of Environment Engineering, Vol. 122, No. 8, pp. 666-673 (1996).
林裕雄,「以電動力法處理受三氯乙烯及單氯酚污染黏質土壤之研究」,碩士論文,國立中興大學環境工程學系,台中(2000)。
翁誌煌,「受有機物污染廠址之物化整治技術研究:電滲透法整治有機污染廠址之研究(第二年)」,行政院國科會專題研究計畫成果報告(1998)。
翁誌煌,陳仁慶,林裕雄,周協裕,「電動力法處理酚類污染土壤之可行性研究」,第十三屆廢棄物處理技術研討會論文集,高雄,第197-198頁(1998)。
翁誌煌,陳仁慶,涂宏旭,林裕雄,袁菁,「電動力復育受單氯酚污染黏質土壤之研究」,第十四屆廢棄物處理技術研討會論文集,中壢,第2-47 ~ 2-54頁(1999)。
翁誌煌、涂宏旭、袁菁,「串聯式電動力法復育受三氯乙烯污染黏質土壤之研究」,第七屆土壤污染整治研討會論文集,台北,第217-232頁 (2001)。
袁菁、翁誌煌、陳威錦、江姿幸,「以複合界面活性劑操作流質提昇電動力技術處理四氯乙烯黏質土壤」,第十六屆廢棄物處理技術研討會論文集光碟,高雄 (2001)。
袁菁、陳威錦、江姿幸,「受苯系有機物污染土壤以電動力-界面活性劑系統處理之研究」,第十五屆廢棄物處理技術研討會論文集,斗六,第2-214 ~ 2-221頁 (2000)。
張坤森,「發展改良式電動力學技術整治鎘污染土壤之研究」,第十三屆廢棄物處理技術研討會論文集,高雄 (1998)。
張坤森、鍾孟儒、吳坦璟、陳南蘋、呂易蒼,「利用超音波及電動力技術促進鎘鉛污染土壤整治之研究」,第十五屆廢棄物處理技術研討會論文集,斗六 (2000a)。
張坤森、羅賢詩、林廷華、葉蕙萍、劉思沁,「以淋洗、超音波及電動力法去除都市垃圾焚化飛灰重金屬之研究」,第十五屆廢棄物處理技術研討會論文集,斗六 (2000b)。
陳政德,「電動力-Fenton法結合生物分解現地處理受五氯酚污染土壤之研究」,碩士論文,國立中山大學環境工程研究所,高雄 (1998)。
章日行,廖盈智,「改良式電動力系統之電化學機制」,第十七屆廢棄物處理技術研討會論文集光碟,台北 (2002)。
斯克誠、駱尚廉,「土壤與地下水污染整治政策與其實務」,土木水利,第26卷,第4期,第50-58頁 (2000)。
楊金鐘、林舜隆,「利用電動力法處理人工合成之鉛污染土壤」,第十一屆廢棄物處理技術研討會論文集,台北,第518-527頁 (1996)。
楊金鐘、陳政德、洪志雄、洪源駿,「電動力-Fenton法處理4-氯酚污染土壤之成效與反應動力討論」,第十五屆廢棄物處理技術研討會論文集,斗六,第2-38 ~ 2-33頁 (2000)。
楊金鐘、劉奇岳,「電動力-Fenton法處理受4-氯酚污染土壤之最佳操作條件探討」,第十四屆廢棄物處理技術研討會論文集,中壢,第2-16 ~ 2-23頁 (1999)。
楊金鐘、龍玉文,「電動力-似Fenton法處理酚、四氯酚砂質壤土之研究」,第十三屆廢棄物處理技術研討會論文集,高雄,第189-196頁 (1998)。
劉永章、葛煥彰,「電動力現象的基本理論」,化工,第四十五卷,第二期,第77-83頁 (1998)。
鄭孟嘉,「以電化學方法處理受鎘、鉛污染土壤之研究」,碩士論文,國立台灣大學化學工程學研究所,台北 (2001)。
龍玉文,「電動力-Fenton法處理受酚與4-氯酚污染土壤之研究」,碩士論文,國立中山大學環境工程研究所,高雄 (1998)。

活動花絮

20120609畢業典禮20120609畢業典禮20120812大學部新生暨家長歡迎會92學畢業紀念冊101學年度畢業典禮102學年度新生茶會與家族聚會
cron web_use_log